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1.
First Ionization Potentials of Fm, Md, No, and Lr: Verification of Filling-Up of 5f Electrons and Confirmation of the Actinide Series / Sato, Tetsuya K (JAEA, Ibaraki) ; Asai, Masato (JAEA, Ibaraki) ; Borschevsky, Anastasia (Groningen U.) ; Beerwerth, Randolf (Jena U., TPI) ; Kaneya, Yusuke (JAEA, Ibaraki) ; Makii, Hiroyuki (JAEA, Ibaraki) ; Mitsukai, Akina (JAEA, Ibaraki) ; Nagame, Yuichiro (JAEA, Ibaraki) ; Osa, Akihiko (JAEA, Ibaraki) ; Toyoshima, Atsushi (JAEA, Ibaraki) et al.
We report the first ionization potentials (IP1) of the heavy actinides, fermium (Fm, atomic number Z = 100), mendelevium (Md, Z = 101), nobelium (No, Z = 102), and lawrencium (Lr, Z = 103), determined using a method based on a surface ionization process coupled to an online mass separation technique in an atom-at-a-time regime. The measured IP1 values agree well with those predicted by state-of-the-art relativistic calculations performed alongside the present measurements. [...]
2018 - 5 p. - Published in : J. Am. Chem. Soc. 140 (2018) 14609-14613 Fulltext: PDF;
2.
First ionization potential of the heaviest actinide lawrencium, element 103 / Sato, Tetsuya K (JAEA, Ibaraki) ; Asai, Masato (JAEA, Ibaraki) ; Borschevsky, Anastasia (Groningen U.) ; Stora, Thierry (CERN ; Gottingen U.) ; Sato, Nozomi (JAEA, Ibaraki) ; Kaneya, Yusuke (JAEA, Ibaraki ; Ibaraki U., Grad. Sch. Sci. Eng.) ; Tsukada, Kazuaki (JAEA, Ibaraki) ; Düllmann, Christoph E (Helmholtz Inst., Mainz ; Darmstadt, GSI ; Mainz U., Inst. Kernphys.) ; Eberhardt, Klaus (Helmholtz Inst., Mainz ; Mainz U., Inst. Kernphys.) ; Eliav, Ephraim (Tel Aviv U.) et al.
The first ionization potential (IP1) of element 103, lawrencium (Lr), has been successfully determined for the first time by using a newly developed method based on a surface ionization process. The measured IP1 value is 4.9630.080.07 eV. [...]
2016 - 6 p. - Published in : EPJ Web Conf. 131 (2016) 05001 Fulltext: PDF;

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