Es1c02165 Si 001
Es1c02165 Si 001
Es1c02165 Si 001
Figure S2. Ecotoxicity(a), human toxicity, cancer (b), human toxicity, non-cancer
(c) of 4 scenarios.
Table S4. Direct gas emissions on nitrification and denitrification processes and
gas combustion.
S2
Figure S1. Description of specific processes and scenarios.
S3
Figure S2. Ecotoxicity(a), human toxicity, cancer (b), human toxicity, non-cancer
(c) of 4 scenarios.
S4
Table S1. Brief description of 7 representative leachate treatment plans (LTPs) surveyed in this study.
MSW* Raw leachate Effluent from MBR Effluent from NF Effluent from RO
Capa
treatmen Locatio Carbon
Name Type city NH3- NO3- BOD NH3- NO3- NH3- NO3- NH3- NO3-
t n Source COD COD COD COD
N N /COD N N N N N N
methods
t/d mg/l mg/l mg/l -- mg/l mg/l mg/l mg/l mg/l mg/l mg/l mg/l mg/l
Waste-
Raw
LTP1 to- Beijing Glucose 900 40000 1800 0 0.3 500 14 900 420 7 900 3 5 30
leachate
energy
Raw
LTP2 Landfill Beijing Glucose 600 10235 3063 0 0.32 1478 17 900 475 8 900 12 0.3 2
leachate
Raw
leachate
LTP3 Landfill Beijing Glucose 1200 5999 2157 5 0.29 1662 6 967 409 4 800 17 1 200
and aged
leacahte
Raw
leachate Methan
LTP4 Landfill Beijing 1000 4454 1210 0 0.21 2130 12 100 333.2 0.97 100 17.7 0.05 20
and aged ol
leacahte
Aged
LTP5 Landfill Shanxi Glucose 200 2500 2200 0 0.1 900 14 200 700 8 200 35 0 40
leacahte
Aged
LTP6 Landfill Sichuan Glucose 1000 10862 2109 10 0.05 1100 5 250 - - - 14 2 10
leacahte
Aged
LTP7 Landfill Sichuan Glucose 1200 11715 2159 10 0.05 1500 5 100 43 1 100 - - -
leacahte
*: Municipal Solid Waste
S5
Table S2. Inventory for operation phase.
S6
HCl 32% kg -- -- 0.06 -- 0.32 0.12 --
NaClO kg 0.05 0.70 -- -- -- -- --
NaOH kg 0.05 -- 0.03 0.03 0.32 -- --
Electricity MJ 10.56 12.82 6.76 16.61 14.26 16.60 --
NaHSO4 kg 0.05 -- -- -- 0.01 -- --
Reverse Osmosis
H3PO4 kg 0.10 0.96 0.02 0.11 0.01 -- --
(RO)
H2SO4 kg -- -- 0.24 -- -- -- --
Operation Inputs for RO concentrate
Natural gas kg 12.55 12.55 12.55 12.55 12.55 15.07 --
Antifoaming agent kg 0.0039 0.0039 0.0039 0.0039 0.0039 0.0047 --
Electricity MJ 14.40 14.40 14.40 14.40 14.40 17.28 --
S7
Table S3. Inventory for construction phase.
Inputs for Construction Phase* (per tonne influent leachate per day)
S8
Stainless steel (304) mg 1193.08 1193.08 1193.08 714.04 750.83 824.18 714.29
Polytetrafluoroethylene (PTFE) mg 16.70 16.70 16.70 10.00 10.51 11.54 10.00
Polyvinylchloride film (PVC) mg 100.22 100.22 100.22 99.97 99.99 100.00 100.00
S9
Construction inputs for major infastructure and equipment
Stainless steel (316) mg 142.85 142.85 142.85 211.14 303.37 395.60 --
Steel rebar mg 4390.00 4390.00 4390.00 4390.00 4390.00 4390.00 --
Cast iron mg 33.00 33.00 33.00 33.00 33.00 33.00 --
S10
Table S4. Direct gas emissions on nitrification and denitrification processes and gas combustion.
Energy alternatives 1
AO+MBR NF RO
Unit Leachate anerobic AO
SCE treatment SCE treatment
(per tonne digestion (N&D*
Scenarios Name (Natural gas combustion) (Natural gas combustion)
influent (Biogas combustion) processes)
leachate)
N2O CH4 N2O CO2 N2O CH4 CO2 N2O CH4
S11
LTP6 g -- -- 55.9 -- -- -- 41916.49 0.07 0.75
Energy alternatives 2
AO+MBR NF RO
Unit Leachate anerobic AO
SCE treatment SCE treatment
(per tonne digestion (N&D*
Scenarios Name (Biogas combustion) Biogas combustion)
influent (Biogas combustion) processes)
leachate)
N2O CH4 N2O N2O CH4 N2O CH4
S13
Table S5. Comparison of three energy supply alternatives.
AP FAETP MAETP Ecotoxicity Human cancer Human non-canc.
-9
Scenario kg SO2 eq. kg DCB eq. kg DCB eq. CTUe CTUh×10 CTUh×10-9
Name
s Alternati Alternati Alternati Alternati Alternati Alternati Alternat Alternati Alternati Alternati Alternati Alternati
ve 1 ve 2 ve 1 ve 2 ve 1 ve 2 ive 1 ve 2 ve 1 ve 2 ve 1 ve 2
LTP1 0.05 0.05 0.12 0.12 2136.46 2136.46 0.01 0.01 1.71 1.71 0.17 0.17
LTP2 0.11 0.11 0.15 0.15 2674.10 2674.10 0.01 0.01 1.99 1.99 0.21 0.21
LTP3 0.08 0.08 0.25 0.25 2554.83 2554.83 0.01 0.01 2.05 2.05 0.19 0.19
Scenario
LTP4 0.09 0.09 0.19 0.19 3426.97 3426.97 0.01 0.01 2.53 2.53 0.26 0.26
2
LTP5 0.09 0.09 0.47 0.47 3340.11 3340.11 0.03 0.03 3.15 3.15 0.25 0.25
LTP6 0.15 0.15 0.89 0.89 5880.62 5880.62 0.03 0.03 4.74 4.74 0.42 0.42
LTP7 0.18 0.18 0.88 0.88 7020.79 7020.79 0.03 0.03 5.33 5.33 0.51 0.51
LTP1 0.08 0.07 0.18 0.16 2861.94 2995.71 0.02 0.01 2.81 2.68 0.22 0.22
LTP2 0.16 0.16 0.23 0.26 3630.83 5461.51 0.03 0.06 3.37 12.15 0.27 0.40
Scenario LTP3 0.10 0.10 0.32 0.35 3278.95 5355.88 0.02 0.06 3.13 13.72 0.25 0.40
3 LTP4 0.12 0.12 0.26 0.29 4219.74 6436.99 0.03 0.06 3.68 14.27 0.33 0.48
LTP5 0.12 0.12 0.53 0.56 4081.26 6298.51 0.04 0.08 4.26 14.85 0.30 0.46
LTP7 0.21 0.21 0.96 1.01 7988.10 10944.43 0.05 0.10 6.68 20.80 0.59 0.80
LTP1 0.13 0.12 0.30 0.33 4350.66 7977.39 0.05 0.09 4.33 20.90 0.34 0.58
LTP2 0.23 0.23 0.37 0.44 5391.57 10673.88 0.07 0.15 5.12 30.40 0.40 0.77
Scenario LTP3 0.15 0.15 0.42 0.51 4549.16 10319.33 0.05 0.14 4.50 32.73 0.35 0.76
4 LTP4 0.18 0.18 0.40 0.48 6024.81 11935.30 0.05 0.15 5.39 33.61 0.47 0.88
LTP5 0.17 0.17 0.66 0.75 5766.58 11677.07 0.07 0.16 5.91 34.13 0.44 0.85
LTP6 0.21 0.21 1.05 1.11 7845.20 12279.61 0.06 0.13 6.66 27.84 0.58 0.89
S14
Human Human non-
EP GWP AP FAETP MAETP Ecotoxicity
cancer canc.
Scenario kg P eq. kg CO2 eq. kg SO2 eq. kg DCB eq. kg DCB eq. CTUe CTUh×10-9 CTUh×10-9
Name
s Alter Alter Alter Alte Alte Alter Alter Alter Alter Alte Alter Alter
Altern Altern Alternat Alternati
nativ nativ nativ rnati rnati nativ nativ nativ nativ rnati native native
ative 1 ative 3 ive 1 ve 3
e1 e3 e1 ve 3 ve 1 e3 e1 e3 e1 ve 3 1 3
Scenario LTP1 1.47 1.47 -- -- -- -- -- -- -- -- -- -- -- -- -- --
1 LTP2 1.24 1.24 -- -- -- -- -- -- -- -- -- -- -- -- -- --
Scenario LTP1 0.12 0.12 32.28 32.28 0.05 0.05 0.12 0.12 2136.46 2136.46 0.01 0.01 1.71 1.71 0.17 0.17
2 LTP2 0.16 0.16 43.62 43.62 0.11 0.11 0.15 0.15 2674.10 2674.10 0.01 0.01 1.99 1.99 0.21 0.21
Scenario LTP1 0.12 0.12 63.66 36.36 0.08 0.07 0.18 0.16 2861.94 2793.95 0.02 0.01 2.81 2.68 0.22 0.22
3 LTP2 0.14 0.14 79.08 74.47 0.16 0.22 0.23 0.23 3630.83 3619.36 0.03 0.03 3.37 3.35 0.27 0.27
Scenario LTP1 0.03 0.03 117.28 87.59 0.13 0.23 0.30 0.28 4350.66 4276.71 0.05 0.03 4.33 4.19 0.34 0.33
4 LTP2 0.04 0.04 135.45 129.18 0.23 0.40 0.37 0.37 5391.57 5372.88 0.07 0.06 5.12 5.08 0.40 0.40
S15
Table S6. Ranges of parameters for uncertainty analysis.
S16
LTP6 0.08 0.12 3.70 19.11 -- -- 74.16 111.24 -- -- 13.28 19.92 -- -- 15.55 19.01
S17
LTP7 -- -- 46.35 67.17 25 60 0.5 5 80 120
LTP1 227.32 403.54 24.61 60.24 1 10 1 10 15 40
LTP2 30.25 77.83 32.13 79.90 5 25 0.1 5 1 20
LTP3 -- -- 16.20 51.27 5 25 0.05 5 150 250
Scenario 4
LTP4 -- -- 25.80 43.95 10 25 0.01 5 10 30
LTP5 -- -- 42.75 70.35 25 40 0 0 20 50
LTP6 -- -- 41.85 60.57 5 25 0.05 5 5 25
S18