Magnetization Curves of A Spin-One Bethe Lattice: PH - V.rrc.c. L MR Wri, Shef/rrld, Sheffield 7Rh. Uk
Magnetization Curves of A Spin-One Bethe Lattice: PH - V.rrc.c. L MR Wri, Shef/rrld, Sheffield 7Rh. Uk
Magnetization Curves of A Spin-One Bethe Lattice: PH - V.rrc.c. L MR Wri, Shef/rrld, Sheffield 7Rh. Uk
PHYSICS
MAGNETIZATION
1985
&~~rtn~~!~tof Ph_v.rrc.c.
L~mr~wri,~of Shef/rrld,
SheffieldS3
12 March
9 September
K.G. CHAKRABORTY
Received
LETTERS
received
7RH.
UK
for publication
24 June 1985
CHiiiikt...,
(1)
ii
where
Ho,i = -JS,
(2)
c
. .. So exp(-/3H)
S{i}
m = c
se
-1
X
c
so
c
qi}
.. . exp(-PH)
(4)
Hi ii = -JSi
Sii - JS;
Si + DS ,
(3)
of Physics,
Basirhat
College,
0.375-9601/85/S
03.30 0 Elsevier Science Publishers B.V.
(North-Holland Physics Publishing Division)
(5)
with
a = exp[-(L2
+ L,)]
b=exp[-(L2
+L3)]
t2exp(K-D)cosh(K-Ll),
(6)
(7)
c=exp[-(LZ
tLj)+D]
t2cosh(Ll),
K=BJ,K=PJ,D=PDlzandL1,L2
given by
(8)
andLgare
exp(2L,)
= (a/b)-l
(9)
exp(2L,)
= (a/~)-~
(10)
exp(2L3)
= (LI/c)~-~
(11)
moment,
4 = tSi> is found
205
PHYSICS LETTERS
9 September 1985
to be
q = (a z + bZ)/(a z + b z + e Z ) .
(12)
10
X exp[(c~ - zcg)Kc]
= [(z - 1) sinh(Kc) - cosh(Kc) + e x p ( - a K c ) ] z - 1 ,
(13)
with K c = J / k B T c , eL = Y ' / J and ct' = D / J z . In the absence of biquadratic exchange this equation reduces
to that of Katsura [3], and also reduces to that of
Obokata and Oguchi [4] if the single-ion anisotropy
is also neglected.
Detailed calculations of the magnetization as given
by eq. (5) have been made for various strengths of the
interactions J, J ' and D and for several coordination
numbers z. Here only the results for z = 6 and J ' / J =
- 1 . 0 5 are presented since these are most interesting
and contact with the work of Chakraborty and
Morita [5] can be made. In fig. 1 the magnetization
as a function of 1/IJJ is shown for various values of ct'.
It is seen that for ~' = 0 the magnetization exhibits an
anti-Curie temperature Tac in addition to the Curie
temperature T C. As - a ' increases, the anti-Curie temperature moves to lower temperatures and the magnetization curve gradually starts to peak on the low temperature side. A t a critical value C~'c,which can be
shown to be - 0 . 0 5 for our choice of c~, the anti-Curie
temperature is predicted to be zero. In this case the
magnetization increases steadily with decreasing temperature from the Curie point, but in a temperature
range extremely close to zero it drops rapidly to zero
a t zero temperature. F o r values o f - t ~ ' greater than
this critical value the magnetization approaches unity
at zero temperature. Although for - a ' only slightly
!
greater than - ~ c the magnetization curve exhibits a
somewhat unfamiliar form, the conventional shape is
reached for relatively small values o f the single-ion
anisotropy (see the upper curve in fig. 1). We have also carried out extensive computations for other values of t~ and other coordination numbers. A full account o f these results will be reported in due course
when other aspects of our work, including a discussion of the quadrupolar m o m e n t and the phase transition are published.
206
O5
kaT/J
Fig. 1. The magnetization, m, as a function of k B T / J for J'/J
= - 1.05 and z = 6. The successive curves from (a) to (b) are
forD/Jz = 0, -0.01, -0.03, -0.05, -0.08, - 0 . 2 and - 0 . 6
respectively. The curve for - 0.05 falls sharply to the origin
at T = 0 from its maximum value shown.
PHYSICS LETTERS
9 September 1985
References
[1] S. Katsura and M. Takizawa, Prog. Theor. Phys. 51
(1974) 82.
[2] Y. Tanaka and N. Ury~, J. Phys. Soc. Japan 50 (1981)
1140.
[3] S. Katsura, J. Phys. A12 (1979) 2087.
[4] T. Obokata and T. Ogucbi, J. Phys. Soc. Japan 25
(1968) 322.
[5] K.G. Chakraborty and T. Morita, Physica 129A (1985)
415.
[6] T. Morita, Physica 83A (1976) 411.
[7] T. Morita, J. Math. Phys. 13 (1972) 115.
[8 ] K. Takahashi and M. Tanaka, J. Phys. Soc. Japan 46
(1979) 1428.
[9] S. Ohkuro and S. Katsura, J. Phys. A13 (1980) 1501.
[10] I. Nagahara, S. Fujiki and S. Katsura, J. Phys. C14
(1981) 3781.
[11] T. Morita and T. Tanaka, Phys. Rev. 145 (1966) 288.
[12] F. Peruggi, J. Phys. A16 (1983) L713.
207