Damping of spin waves and singularity of the longitudinal modes in the dipolar critical regime of the Heisenberg ferromagnet EuS

P. Böni, B. Roessli, D. Görlitz, and J. Kötzler
Phys. Rev. B 65, 144434 – Published 2 April 2002
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Abstract

By inelastic scattering of polarized neutrons near the (200) Bragg reflection, the susceptibilities and linewidths of the spin waves and the longitudinal spin fluctuations, δSsw(q) and δSz(q)Ms, respectively, were determined separately. By aligning the momentum transfers q perpendicular to both δSsw and the spontaneous magnetization Ms, we explored the statics and dynamics of these modes with transverse polarizations with respect to q. In the dipolar critical regime, where the inverse correlation length κz(T) and q are smaller than the dipolar wave number qd, we observe that (i) the static susceptibility of δSswt(q) displays the Goldstone divergence while for δSzt(q) the Ornstein-Zernicke shape fits the data with a possible indication of a thermal (mass) renormalization at the smallest q values; i.e., we find indications for the predicted 1/q divergence of the longitudinal susceptibility; (ii) the spin-wave dispersion as predicted by the Holstein-Primakoff theory revealing qd=0.23(1)Å1, in good agreement with previous work in the paramagnetic and ferromagnetic regime of EuS; (iii) within experimental error, the (Lorentzian) linewidths of both modes turn out to be identical with respect to the q2 variation, the temperature independence, and the absolute magnitude. Due to the linear dispersion of the spin waves, they remain underdamped for q<qd. These central results differ significantly from the well-known exchange-dominated critical dynamics, but are quantitatively explained in terms of dynamical scaling and existing data for T>~TC. The available mode-mode coupling theory, which takes the dipolar interactions fully into account, describes the gross features of the linewidths but not all details of the T and q dependences.

  • Received 18 October 2001

DOI:https://doi.org/10.1103/PhysRevB.65.144434

©2002 American Physical Society

Authors & Affiliations

P. Böni

  • Physik-Department E21, Technische Universität München, D-85748 Garching, Germany
  • Laboratory for Neutron Scattering ETH & PSI, CH-5232 Villigen PSI, Switzerland

B. Roessli

  • Institut Laue Langevin, F-38042 Grenoble, France
  • Laboratory for Neutron Scattering ETH & PSI, CH-5232 Villigen PSI, Switzerland

D. Görlitz and J. Kötzler*

  • Institut für Angewandte Physik und Zentrum für Mikrostrukturforschung, D-20355 Hamburg, Germany

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Vol. 65, Iss. 14 — 1 April 2002

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