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Temperature Dependence of the Hyperfine Magnetic Field at Fe Sites in Ba-Doped BiFeO$_3$ Thin Films Studied by Emission Mössbauer Spectroscopy
/ Heiniger-Schell, Juliana (CERN ; Duisburg-Essen U.) ; Bharuth-Ram, Krish (ENS, Lyon, Lab. Phys. ; KwaZulu Natal U. ; DUT, Durban) ; Naicker, Kimara (ENS, Lyon, Lab. Phys. ; KwaZulu Natal U.) ; Masondo, Vusumuzi (DUT, Durban) ; Dang, Thien Thanh (Duisburg-Essen U.) ; Escobar, Marianela (Duisburg-Essen U.) ; Díaz-Guerra, Carlos (Madrid U.) ; Marschick, Georg (Vienna, Tech. U.) ; Masenda, Hilary (Witwatersrand U.) ; Gunnlaugsson, Haraldur P (Iceland U.) et al.
Emission $^{57}$Fe Mössbauer spectroscopy (eMS), following the implantation of radioactive $^{57}$Mn+ ions, has been used to study the temperature dependence of the hyperfine magnetic field at Fe sites in Ba-doped BiFeO$_3$ (BFO) thin films. $^{57}$Mn β decays (t$_{1/2}$ = 90 s) to the 14.4 keV Mössbauer state of $^{57}$Fe, thus allowing online eMS measurements at a selection of sample temperatures during Mn implantation. [...]
2023 - 13 p.
- Published in : Crystals 13 (2023) 724
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Magnetic origins of epitaxial MAX phase Mn2GaC-based thin films probed by Emission Mössbauer Spectroscopy
/ Qi, Bingcui (Science Institute, University of Iceland, Iceland) ; Gunnlaugsson, Haraldur Páll (Science Institute, University of Iceland, Iceland) ; Ólafsson, Sveinn (Science Institute, University of Iceland, Iceland) ; Þorsteinsson, Einar Baldur (Science Institute, University of Iceland, Iceland) ; Magnus, Friðrik (Science Institute, University of Iceland, Iceland) ; Rosén, Johanna (Materials Design Division, Department of Physics, Chemistry and Biology, IFM, Linköping University, Linköping 58183, Sweden) ; Tao, Quanzheng (Materials Design Division, Department of Physics, Chemistry and Biology, IFM, Linköping University, Linköping 58183, Sweden) ; Mantovan, Roberto (3CNR-IMM, Unit of Agrate Brianza, Via C. Olivetti 2, 20864 Agrate Brianza (MB), Italy) ; Masenda, Hilary (School of Physics, University of the Witwatersrand, South Africa) ; Zyabkin, Dmitry (Ilmenau, Gustav-Kirchhoff-Strasse 5, 98693 Ilmenau, Germany) et al.
CERN-INTC-2024-017 ; INTC-P-696.
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2024.
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Compositional Dependence of Epitaxial
L
1
0
‐Mn
x
Ga Magnetic Properties as Probed by
57
Mn/Fe and
119
In/Sn Emission Mössbauer Spectroscopy
/ Unzueta, Iraultza (Basque U., Bilbao) ; Gunnlaugsson, Haraldur Pall (Iceland U.) ; Mølholt, Torben Esmann (CERN) ; Masenda, Hilary (U. Witwatersrand, Johannesburg, Sch. Phys.) ; Mokhles Gerami, Adeleh (IPM, Tehran) ; Krastev, Petko (Sofiya, Inst. Nucl. Res.) ; Zyabkin, Dmitry V (Ilmenau Tech. U.) ; Bharuth-Ram, Krish (KwaZulu Natal U.) ; Naidoo, Deena (U. Witwatersrand, Johannesburg, Sch. Phys.) ; Ólafsson, Sveinn (Iceland U.) et al.
The magnetic properties of MnxGa alloys critically depend on compositionx, andthe atomic-scale origin of those dependences is still not fully disclosed. Molecularbeam epitaxy has been used to produce a set of MnxGa samples (x¼0.7÷1.9)with strong perpendicular magnetic anisotropy, and controllable saturationmagnetization and coercivefield depending onx. [...]
2022 - 11 p.
- Published in : Phys. Status Solidi B 259 (2022) 2200121
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Anisotropy of the Electric Field Gradient in Two-Dimensional α-MoO$_3$ Investigated by $^{57}$Mn($^{57}$Fe) Emission Mössbauer Spectroscopy
/ Schell, Juliana (CERN ; Duisburg-Essen U.) ; Zyabkin, Dmitry (Ilmenau Tech. U.) ; Bharuth-Ram, Krish (KwaZulu Natal U.) ; Gonçalves, João N (Aveiro U.) ; Díaz-Guerra, Carlos (Madrid U.) ; Gunnlaugsson, Haraldur P (Iceland U.) ; Martín-Luengo, Aitana Tarazaga (Linz U.) ; Schaaf, Peter (Ilmenau Tech. U.) ; Bonanni, Alberta (Linz U.) ; Masenda, Hilary (Witwatersrand U. ; Philipps U. Marburg) et al.
Van der Waals α-MoO3 samples offer a wide range of attractive catalytic, electronic, and optical properties. We present herein an emission Mössbauer spectroscopy (eMS) study of the electric-field gradient (EFG) anisotropy in crystalline free-standing α-MoO3 samples. [...]
2022 - 13 p.
- Published in : Crystals 12 (2022) 942
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Confirming the Unusual Temperature Dependence of the Electric-Field Gradient in Zn
/ Haas, Heinz (Aveiro U. ; CERN) ; Zyabkin, Dmitry (Ilmenau Tech. U.) ; Schell, Juliana (CERN ; Duisburg-Essen U.) ; Dang, Thien T (Duisburg-Essen U.) ; Yap, Ian C J (Gottingen U., II. Phys. Inst.) ; Michelon, Ilaria (Padua U.) ; Gaertner, Daniel (Munster U.) ; Gerami, Adeleh Mokhles (IPM, Tehran) ; Noll, Cornelia (Bonn U.) ; Beck, Reinhard (Bonn U.)
The electric-field gradient (EFG) at nuclei in solids is a sensitive probe of the charge distribution. Experimental data, which previously only existed in insulators, have been available for metals with the development of nuclear measuring techniques since about 1970. [...]
2022 - 8 p.
- Published in : Crystals 12 (2022) 1064
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Charge and spin state of dilute Fe in NaCl and LiF
/ ISOLDE Collaboration
There is an apparent mismatch between electron paramagnetic resonance and Mössbauer spectroscopy results on the charge and spin states of dilute Fe impurities in NaCl; Mössbauer spectroscopy data have been interpreted in terms of high-spin Fe$^{2+}$, while electron paramagnetic resonance studies suggest low-spin Fe$^{1+}$. In the present study, the charge and spin states of dilute substitutional Fe impurities in NaCl and LiF have been investigated with $^{57}$Mn → $^{57}$Fe emission Mössbauer spectroscopy. [...]
2022 - 10 p.
- Published in : Phys. Rev. B 106 (2022) 174108
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Temperature dependence of the local electromagnetic field at the Fe site in multiferroic bismuth ferrite
/ Dang, T T (U. Duisburg-Essen) ; Schell, J (U. Duisburg-Essen ; CERN) ; Boa, A G (Denmark, Tech. U.) ; Lewin, D (U. Duisburg-Essen) ; Marschick, G (TU Vienna) ; Dubey, A (U. Duisburg-Essen) ; Escobar-Castillo, M (Duisburg-Essen U.) ; Noll, C (Bonn U., HISKP) ; Beck, R (Bonn U., HISKP) ; Zyabkin, Dmitry V (Ilmenau Tech. U.) et al.
In this paper, we present a study of the temperature-dependent characteristics of electromagnetic fields at the atomic scale in multiferroic bismuth ferrite (BiFeO$_3$ or BFO). The study was performed using time differential perturbed angular correlation (TDPAC) spectroscopy on implanted 111In (111Cd) probes over a wide temperature range. [...]
2022 - 15 p.
- Published in : Phys. Rev. B 106 (2022) 054416
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Metal-insulator transition in crystalline V$_2$O$_3$ thin films probed at atomic-scale using emission Mössbauer spectroscopy
/ Qi, B (Iceland U.) ; Gunnlaugsson, H P (Iceland U.) ; Ólafsson, S (Iceland U.) ; Gislason, H P (Iceland U.) ; Thorsteinsson, E B (Iceland U.) ; Arnalds, U B (Iceland U.) ; Mantovan, R (CNR-IMM, Catania) ; Unzueta l, I (Basque U., Bilbao) ; Zyabkin, D V (Ilmenau Tech. U.) ; Bharuth Ram, K (KwaZulu Natal U. ; DUT, Durban) et al.
Microscopic understanding the metal-to-insulator transition (MIT) in strongly correlated materials is critical to
the design and control of modern “beyond silicon” Mott nanodevices. In this work, the local MIT behaviors in
single crystalline V$_2$O$_3$ thin films were probed on an atomic scale by online $^{57}$Fe emission Mössbauer spectroscopy (eMS) following dilute ($<10^{-3}$ at.%) implantation of $^{57}$Mn$^+$ (T$_{1/2}$ = 90 s). [...]
2020
- Published in : Thin Solid Films 714 (2020) 138389
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10.
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Experimental and Theoretical Study of Electronic and Hyperfine Properties of Hydrogenated Anatase (TiO2): Defect Interplay and Thermal Stability
/ Zyabkin, D V (Palacky U. ; Ilmenau Tech. U.) ; Gunnlaugsson, H P (Iceland U.) ; Gonçalves, J N (Aveiro U.) ; Bharuth-Ram, K (KwaZulu Natal U. ; DUT, Durban) ; Qi, B (Iceland U.) ; Unzueta, I (Basque U., Bilbao) ; Naidoo, D (Witwatersrand U.) ; Mantovan, R (CNR-IMM, Catania) ; Masenda, H (Witwatersrand U.) ; Ólafsson, S (Iceland U.) et al.
The performance of TiO$_2$-based materials is highly dependent on the electronic structure and local defect configurations. Hence, a thorough understanding of defect interaction plays a key role. [...]
2020 - 12 p.
- Published in : The Journal of Physical Chemistry C 124 (2020) 7511-7522
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