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Ionization potential of radium monofluoride / Wilkins, S.G. (MIT) ; Perrett, H.A. (Manchester U.) ; Udrescu, S.M. (MIT) ; Kyuberis, A.A. (U. Groningen, VSI) ; Pašteka, L.F. (U. Groningen, VSI ; Comenius U.) ; Au, M. (CERN ; Mainz U.) ; Belošević, I. (MIT ; TRIUMF) ; Berger, R. (Philipps U. Marburg) ; Binnersley, C.L. (Manchester U.) ; Bissell, M.L. (Manchester U.) et al.
The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. [...]
arXiv:2408.14673. - 10.
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Precision spectroscopy and laser-cooling scheme of a radium-containing molecule / Udrescu, S M (MIT) ; Wilkins, S G (MIT) ; Breier, A A (Kassel U.) ; Athanasakis-Kaklamanakis, M (CERN ; Leuven U.) ; Ruiz, R F Garcia (MIT) ; Au, M (CERN ; Mainz U.) ; Belošević, I (TRIUMF) ; Berger, R (Philipps U. Marburg) ; Bissell, M L (Manchester U.) ; Binnersley, C L (Manchester U.) et al.
Molecules containing heavy radioactive nuclei are predicted to be extremely sensitive to violations of the fundamental symmetries of nature. The nuclear octupole deformation of certain radium isotopes massively boosts the sensitivity of radium monofluoride molecules to symmetry-violating nuclear properties. [...]
2024 - 14 p. - Published in : Nature Phys. 20 (2024) 202-207

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Radiative lifetime of the A 2Π1/2 state in RaF with relevance to laser cooling / ISOLDE Collaboration
The radiative lifetime of the $A$$^2 \Pi_{1/2}$ (v=0) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate $\Gamma = 2.86(8) \times 10^7$$s^{-1}$ are of relevance to the laser cooling of RaF via the optically closed $A$$^2 \Pi_{1/2} \leftarrow X$$^2\Sigma_{1/2}$ transition, which makes the molecule a promising probe to search for new physics. [...]
arXiv:2403.09336.- 2024-07-22 - 8 p. - Published in : Phys. Rev. A 110 (2024) L010802 Fulltext: PDF;

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Pinning down electron correlations in RaF via spectroscopy of excited states / ISOLDE Collaboration
We report the spectroscopy of 11 electronic states in the radioactive molecule radium monofluoride (RaF). [...]
arXiv:2308.14862. - 18 p.
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Observation of the distribution of nuclear magnetization in a molecule / Wilkins, S.G. (MIT) ; Udrescu, S.M. (MIT) ; Athanasakis-Kaklamanakis, M. (CERN ; Leuven U.) ; Garcia Ruiz, R.F. (MIT) ; Au, M. (CERN ; Mainz U.) ; Belošević, I. (TRIUMF) ; Berger, R. (Philipps U. Marburg) ; Bissell, M.L. (Manchester U.) ; Breier, A.A. (Kassel U.) ; Brinson, A.J. (MIT) et al.
Rapid progress in the experimental control and interrogation of molecules, combined with developments in precise calculations of their structure, are enabling new opportunities in the investigation of nuclear and particle physics phenomena. [...]
arXiv:2311.04121. -
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King-Plot Analysis of Isotope Shifts in Simple Diatomic Molecules / Athanasakis-Kaklamanakis, Michail (CERN ; Leuven U.) ; Wilkins, Shane G. (MIT) ; Breier, Alexander A. (Kassel U.) ; Neyens, Gerda (Leuven U.)
We demonstrate that the isotope shift in isotopomers of diatomic molecules, where the nucleus of one of its constituent atoms is replaced by another isotope, can be expressed as the sum of a field shift and a mass shift, similar to the atomic case. We show that a linear relation holds between atomic and molecular isotopes shifts, thus extending the King-plot analysis to molecular isotope shifts. [...]
arXiv:2301.11064.- 2023-01-01 - 17 p. - Published in : Phys. Rev. X: 13 (2023) , no. 1, pp. 011015 Fulltext: 2301.11064 - PDF; Publication - PDF;

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Opportunities for Fundamental Physics Research with Radioactive Molecules / Arrowsmith-Kron, Gordon (Michigan State U.) ; Athanasakis-Kaklamanakis, Michail (CERN ; Leuven U.) ; Au, Mia (CERN ; Mainz U.) ; Ballof, Jochen (CERN ; Michigan State U.) ; Berger, Robert (Philipps U. Marburg) ; Borschevsky, Anastasia (U. Groningen, VSI) ; Breier, Alexander A. (Kassel U.) ; Buchinger, Fritz (McGill U.) ; Budker, Dmitry (Darmstadt, GSI ; UC, Berkeley) ; Caldwell, Luke (JILA, Boulder ; U. Colorado, Boulder ; Colorado U.) et al.
Molecules containing short-lived, radioactive nuclei are uniquely positioned to enable a wide range of scientific discoveries in the areas of fundamental symmetries, astrophysics, nuclear structure, and chemistry. Recent advances in the ability to create, cool, and control complex molecules down to the quantum level, along with recent and upcoming advances in radioactive species production at several facilities around the world, create a compelling opportunity to coordinate and combine these efforts to bring precision measurement and control to molecules containing extreme nuclei. [...]
arXiv:2302.02165.- 2024-07-12 - 119 p. - Published in : Rep. Prog. Phys. 87 (2024) 084301 Fulltext: PDF;

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Isotope Shifts of Radium Monofluoride Molecules / Udrescu, S.M. (MIT) ; Brinson, A.J. (MIT) ; Ruiz, R.F. Garcia (MIT ; CERN) ; Gaul, K. (Philipps U. Marburg) ; Berger, R. (Philipps U. Marburg) ; Billowes, J. (Manchester U.) ; Binnersley, C.L. (Manchester U.) ; Bissell, M.L. (Manchester U.) ; Breier, A.A. (Kassel U.) ; Chrysalidis, K. (CERN) et al.
Isotope shifts of $^{223-226,228}$Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^{2}{}{\Pi}_{1/2}\leftarrow X^{2}{}{\Sigma}^{+}$. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. [...]
arXiv:2105.10549.- 2021-07-14 - 7 p. - Published in : Phys. Rev. Lett. 127 (2021) 033001 Fulltext: 2105.10549 - PDF; PhysRevLett.127.033001 - PDF; Fulltext from publisher: PDF;

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Spectroscopy of short-lived radioactive molecules / Garcia Ruiz, R.F. (CERN ; MIT) ; Breier, A.A. (Kassel U.) ; Giesen, T.F. (Kassel U.) ; Koszorús, Á. (Leuven U.) ; Berger, R. (Unlisted, DE) ; Billowes, J. (Manchester U.) ; Binnersley, C.L. (Manchester U.) ; Bissell, M.L. (Manchester U.) ; Brinson, A.J. (MIT) ; Chrysalidis, K. (CERN) et al.
The study of molecular systems provides exceptional opportunities for the exploration of the fundamental laws of nature and for the search for physics beyond the Standard Model of particle physics. Measurements of molecules composed of naturally occurring nuclei have provided the most stringent upper bounds to the electron electric dipole moment to date, and offer a route to investigate the violation of fundamental symmetries with unprecedented sensitivity. [...]
arXiv:1910.13416.- 2020-05-27 - 10 p. - Published in : Nature 581 (2020) 396-400 Fulltext: PDF; Fulltext from Publisher: PDF;

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10.

ISOLDE PROGRAMME / Zakoucky, D

et al.
Approved: 19 December 1964.-
Status: Data Taking
External link: Experiment home page
Experiment: ISOLDE

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6	Breier, A.A.
2	Breier, Alexander A.

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