CERN Accelerating science

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1.
Effect of ions on sulfuric acid-water binary particle formation: 1. Theory for kinetic- and nucleation-type particle formation and atmospheric implications / Merikanto, Joonas (Helsinki Inst. of Phys. ; Finnish Meteorological Inst.) ; Duplissy, Jonathan (Helsinki U. ; Helsinki Inst. of Phys.) ; Määttänen, Anni (Versailles U., Velizy ; LATMOS, Guyancourt ; Paris U., IV) ; Henschel, Henning (Helsinki U.) ; Donahue, Neil M (Carnegie Mellon U.) ; Brus, David (Finnish Meteorological Inst.) ; Schobesberger, Siegfried (Helsinki Inst. of Phys.) ; Kulmala, Markku (Helsinki U.) ; Vehkamäki, Hanna (Helsinki Inst. of Phys.)
We derive a version of Classical Nucleation Theory normalized by quantum chemical results on sulfuric acid-water hydration to describe neutral and ion-induced particle formation in the binary sulfuric acid-water system. The theory is extended to treat the kinetic regime where the nucleation free energy barrier vanishes at high sulfuric acid concentrations or low temperatures. [...]
2016 - 16 p. - Published in : J. Geophys. Res. 121 (2016) 1736-1751
2.
Effect of ions on sulfuric acid-water binary particle formation: 2. Experimental data and comparison with QC-normalized classical nucleation theory / Duplissy, J. ; Merikanto, J. ; Franchin, A. ; Tsagkogeorgas, G. ; Kangasluoma, J. ; Wimmer, D. ; Vuollekoski, H. ; Schobesberger, S. ; Lehtipalo, K. ; Flagan, R. C. et al.
We report comprehensive, demonstrably contaminant‐free measurements of binary particle formation rates by sulfuric acid and water for neutral and ion‐induced pathways conducted in the European Organization for Nuclear Research Cosmics Leaving Outdoor Droplets chamber. The recently developed Atmospheric Pressure interface‐time of flight‐mass spectrometer was used to detect contaminants in charged clusters and to identify runs free of any contaminants. [...]
2015-09-04 - 24 p. - Published in : J. Geophys. Res. Atmos. 121 (2016) 1752-1775 External link: Fulltext
3.
Global atmospheric particle formation from CERN CLOUD measurements / Dunne, E M (Leeds U.) ; Gordon, H (CERN) ; Kurten, A ; Almeida, J ; Duplissy, J ; Williamson, C ; Ortega, I K ; Pringle, K J ; Adamov, A ; Baltensperger, U et al. /CLOUD
Fundamental questions remain about the origin of newly formed atmospheric aerosol particles because data from laboratory measurements have been insufficient to build global models. In contrast, gas-phase chemistry models have been based on laboratory kinetics measurements for decades. [...]
2016 - 6 p. - Published in : Science 354 (2016) 1119-1124

似た著者名:
1 Merikanto, J
1 Merikanto, Joonas
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