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Radiative Decay of the $^{229m}$Th Nuclear Clock Isomer in Different Host Materials
/ Pineda, S.V. (Leuven U.) ; Chhetri, P. (Leuven U. ; Mainz U.) ; Bara, S. (Leuven U.) ; Elskens, Y. (Leuven U.) ; Casci, S. (Leuven U.) ; Alexandrova, A.N. (UCLA, Los Angeles (main)) ; Au, M. (CERN) ; Athanasakis-Kaklamanakis, M. (Leuven U. ; CERN ; Imperial Coll., London) ; Bartokos, M. (Vienna, Tech. U., Atominst.) ; Beeks, K. (Ecole Polytechnique, Lausanne) et al.
A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the $^{229m}$Th nuclear clock isomer embedded in different host materials is reported. [...]
arXiv:2408.12309.
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As$^{\textrm{III}}$ Selectively Induces a Disorder-to-Order Transition in the Metalloid Binding Region of the AfArsR Protein
/ Tóth, Annamária ; Sajdik, Kadosa ; Gyurcsik, Béla ; Nafaee, Zeyad H ; Wéber, Edit ; Kele, Zoltan ; Christensen, Niels Johan ; Schell, Juliana (CERN) ; Correia, Joao Guilherme (CERN) ; Clauss, Kajsa G V Sigfridsson et al.
Arsenic is highly toxic and a significant threat to human health, but certain bacteria have developed defense mechanisms initiated by AsIII binding to AsIII-sensing proteins of the ArsR family. The transcriptional regulator AfArsR responds to AsIII and SbIII by coordinating the metalloids with three cysteines, located in a short sequence of the same monomer chain. [...]
2024 - 14 p.
- Published in : J. Am. Chem. Soc. 146 (2024) 17009-17022
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Structural formation yield of GeV centers from implanted Ge in diamond
/ Wahl, Ulrich (IST, Lisbon (main)) ; Correia, João Guilherme (IST, Lisbon (main)) ; Costa, Ângelo (Leuven U.) ; Lamelas, Afonso (Aveiro U.) ; Amaral, Vítor (Aveiro U.) ; Johnston, Karl (CERN) ; Magchiels, Goele (Leuven U.) ; Tunhuma, Shandirai Malven (Leuven U.) ; Vantomme, André (Leuven U.) ; Pereira, Lino M C (Leuven U.)
In order to study the structural formation yield of germanium-vacancy (GeV) centers from implanted Ge in diamond, we have investigated its lattice location by using the β$^{−}$ emission channeling technique from the radioactive isotope $^{75}$Ge (t$_{1/2}$ = 83 min) produced at the ISOLDE/CERN facility. $^{75}$Ge was introduced via recoil implantation following 30 keV ion implantation of the precursor isotope $^{75}$Ga (126 s) with fluences around 2 × 10$^{12}$–5 × 10$^{13}$ cm$^{−2}$. [...]
2024 - 16 p.
- Published in : Mat. Quant. Tech. 4 (2024) 025101
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The EFG at Hg and Cd for isolated molecules in frozen solution
/ Röder, J (Aveiro U. ; CERN) ; Haas, H (Aveiro U. ; CERN) ; Correia, J G (CERN ; Lisbon, IST) ; van Stiphout, K (Gottingen U., II. Phys. Inst.)
In order to obtain quantitative information about the changes of the EFG in closed-shell metal-organic molecules by the interactions with an inert matrix, two cases, dimethylmercury and dimethylcadmium, were measured using $^{199m}$Hg and $^{111m}$Cd PAC, respectively, in frozen diethyl ether and tetrahydrofuran. With the knowledge of high-accuracy nuclear quadrupole moments and available precision EFG values from quantum chemistry CCSD-T calculations the expected NQI frequencies of the free molecules are available and can be compared to the ones measured in the frozen solutions..
2024 - 6 p.
- Published in : Hyperfine Interact. 245 (2024) 48
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Magnesium-Vacancy Optical Centers in Diamond
/ Corte, Emilio ; Andrini, Greta ; Nieto Hernández, Elena ; Pugliese, Vanna ; Costa, Ângelo ; Magchiels, Goele ; Moens, Janni ; Tunhuma, Shandirai Malven ; Villarreal, Renan ; Pereira, Lino M. C. et al.
We provide the first systematic characterization of the structural and photoluminescence properties of optically active centers fabricated upon implantation of 30–100 keV Mg+ ions in synthetic diamond. The structural configurations of Mg-related defects were studied by the electron emission channeling technique for short-lived, radioactive 27Mg implantations at the CERN-ISOLDE facility, performed both at room temperature and 800 °C, which allowed the identification of a major fraction of Mg atoms (∼30 to 42%) in sites which are compatible with the split-vacancy structure of the MgV complex. [...]
- Published in : ACS Photonics 10 (2023) 101-110
Fulltext: MgV_SupportingInformation - PDF; ACSPhotonics_2023_10_0101 - PDF;
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Cd implantation in α-MoO3: An atomic scale study
/ Gerami, Adeleh Mokhles (IPM, Tehran ; CERN) ; Heiniger-Schell, Juliana (CERN ; Duisburg-Essen U.) ; da Silva, E Lora (Porto U.) ; Costa, Messias S (Para U.) ; Costa, Cleidilane S (Para U.) ; Monteiro, João G (IST/ITN, Lisbon) ; Pires, José J (Lisbon, CFTP) ; Pereira, Daniela R (Lisbon, ISEL) ; Díaz-Guerra, Carlos (Madrid U.) ; Carbonari, Artur W (IPEN, Sao Paulo) et al.
Lamellar α-MoO3 crystals were implanted with low fluence of radioactive Cd111m ions at ISOLDE-CERN. Subsequently, we have probed the interaction of the Cd impurity in the lattice with native point defects, such as oxygen vacancies, as a function of annealing temperature using the time differential perturbed angular correlations nanoscopic technique. [...]
2023 - 15 p.
- Published in : Phys. Rev. Mater. 7 (2023) 033603
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Microscopic insight by nuclear hyperfine methods on ferroic Perovskites
/ Lopes, A M L ; Schell, J H ; Carbonari, A W ; Amaral, V S ; Araujo, J P ; Lupascu, D C ; Dang, T T ; Yap, I C J ; Burimova, A ; Correia, J G et al.
CERN-INTC-2023-045 ; INTC-CLL-054.
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Fulltext - Original Document (INTC-P-663)
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Probing structural transitions in M(II) vanadates (M = Zn, Mn, Cd, Ca) with TDPAC spectroscopy
/ Burimova, Anastasia (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Carbonari, Artur Wilson (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Heiniger-Schell, Juliana (European Organization for Nuclear Research (CERN), CH-1211 Geneva, Switzerland; Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen, 45141 Essen, Germany) ; Leite Neto, Osmar Flavio da Silveira (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Saxena, Rajendra Narain (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Sales, Tatiane da Silva Nascimento (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Genezini, Frederico Antonio (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Pereira, Luciano Fabricio Dias (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Ribeiro Junior, Ibere Souza (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) ; Correa, Bruno Santos (Instituto de Pesquisas Energeticas e Nucleares, IPEN, Sao Paulo, SP, Brazil) et al.
CERN-INTC-2023-023 ; INTC-P-661.
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