Bräkling, Steffen - Résultats de la recherche

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An intercomparison study of four different techniques for measuring the chemical composition of nanoparticles / Caudillo, Lucía (Frankfurt U., FIAS ; Frankfurt U.) ; Surdu, Mihnea (PSI, Villigen) ; Lopez, Brandon (Carnegie Mellon U.) ; Wang, Mingyi (Carnegie Mellon U. ; Caltech) ; Thoma, Markus (Frankfurt U., FIAS ; Frankfurt U.) ; Bräkling, Steffen (LLNL, Livermore) ; Buchholz, Angela (Aalto U.) ; Simon, Mario (Frankfurt U., FIAS ; Frankfurt U.) ; Wagner, Andrea C (Frankfurt U., FIAS ; Frankfurt U.) ; Müller, Tatjana (Frankfurt U., FIAS ; Frankfurt U. ; Mainz, Max Planck Inst.) et al.
Currently, the complete chemical characterization of nanoparticles (< 100 nm) represents an analytical challenge, since these particles are abundant in number but have negligible mass. Several methods for particle-phase characterization have been recently developed to better detect and infer more accurately the sources and fates of sub-100 nm particles, but a detailed comparison of different approaches is missing. Here we report on the chemical composition of secondary organic aerosol (SOA) nanoparticles from experimental studies of α-pinene ozonolysis at −50, −30, and −10 ∘C and intercompare the results measured by different techniques. [...]
2023 - 19 p. - Published in : Atmos. Chem. Phys. 23 (2023) 6613-6631 Fulltext: PDF;

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Enhanced growth rate of atmospheric particles from sulfuric acid / Stolzenburg, Dominik (Vienna U. ; Helsinki U.) ; Simon, Mario (Frankfurt U.) ; Ranjithkumar, Ananth (Leeds U.) ; Kürten, Andreas (Frankfurt U.) ; Lehtipalo, Katrianne (Helsinki U. ; Finnish Meteorological Inst.) ; Gordon, Hamish (Leeds U.) ; Ehrhart, Sebastian (Mainz, Max Planck Inst.) ; Finkenzeller, Henning (U. Colorado, Boulder) ; Pichelstorfer, Lukas (Helsinki U.) ; Nieminen, Tuomo (Helsinki U.) et al.
In the present-day atmosphere, sulfuric acid is the most important vapour for aerosol particle formation and initial growth. However, the growth rates of nanoparticles ( < 10 nm) from sulfuric acid remain poorly measured. [...]
2020 - 14 p. - Published in : Atmos. Chem. Phys. 20 (2020) 7359-7372

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Molecular understanding of new-particle formation from $\alpha$-pinene between −50 and +25 °C / Simon, Mario (Frankfurt U.) ; Dada, Lubna (Helsinki U.) ; Heinritzi, Martin (Frankfurt U.) ; Scholz, Wiebke (Innsbruck U.) ; Stolzenburg, Dominik (Vienna U.) ; Fischer, Lukas (Innsbruck U.) ; Wagner, Andrea C (Frankfurt U. ; U. Colorado, Boulder) ; Kürten, Andreas (Frankfurt U.) ; Rörup, Birte (Helsinki U.) ; He, Xu-Cheng (Helsinki U.) et al.
Highly oxygenated organic molecules (HOMs) contribute substantially to the formation and growth of atmospheric aerosol particles, which affect air quality, human health and Earth’s climate. HOMs are formed by rapid, gasphase autoxidation of volatile organic compounds (VOCs) such as α-pinene, the most abundant monoterpene in the atmosphere. [...]
2020 - 25 p. - Published in : Atmos. Chem. Phys. 20 (2020) 9183-9207

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Measurement of ammonia, amines and iodine compounds using protonated water cluster chemical ionization mass spectrometry / Pfeifer, Joschka (CERN ; Goethe U., Frankfurt (main)) ; Simon, Mario (Goethe U., Frankfurt (main)) ; Heinritzi, Martin (Goethe U., Frankfurt (main)) ; Piel, Felix (Goethe U., Frankfurt (main)) ; Weitz, Lena (Goethe U., Frankfurt (main)) ; Wang, Dongyu (PSI, Villigen) ; Granzin, Manuel (Goethe U., Frankfurt (main)) ; Müller, Tatjana (Goethe U., Frankfurt (main)) ; Bräkling, Steffen (Unlisted, CH) ; Kirkby, Jasper (CERN ; Goethe U., Frankfurt (main)) et al.
Here we describe the design and performance of a new water cluster chemical ionization–atmospheric pressure interface time-of-flight mass spectrometer (CI-APi-TOF). The instrument selectively measures trace gases with high proton affinity such as ammonia and dimethylamine, which are important for atmospheric new particle formation and growth. [...]
2020 - 22 p. - Published in : Atmos. Meas. Tech. 13 (2020) 2501-2522 Fulltext from Publisher: PDF;

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Rapid growth of new atmospheric particles by nitric acid and ammonia condensation / Wang, Mingyi (Carnegie Mellon U.) ; Kong, Weimeng (Caltech) ; Marten, Ruby (PSI, Villigen) ; He, Xu-Cheng (Helsinki U.) ; Chen, Dexian (Carnegie Mellon U.) ; Pfeifer, Joschka (CERN) ; Heitto, Arto (Kuopio U.) ; Kontkanen, Jenni (Helsinki U.) ; Dada, Lubna (Helsinki U.) ; Kürten, Andreas (Goethe U., Frankfurt (main)) et al.
Measurements in the CLOUD chamber at CERN show that the rapid condensation of ammonia and nitric acid vapours could be important for the formation and survival of new particles in wintertime urban conditions, contributing to urban smog..
2020 - 20 p. - Published in : Nature 581 (2020) 184-189 Fulltext from Publisher: PDF;

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