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Title First ionization potential of the heaviest actinide lawrencium, element 103
Author(s) Sato, Tetsuya K (JAEA, Ibaraki) ; Asai, Masato (JAEA, Ibaraki) ; Borschevsky, Anastasia (Groningen U.) ; Stora, Thierry (CERN ; Gottingen U.) ; Sato, Nozomi (JAEA, Ibaraki) ; Kaneya, Yusuke (JAEA, Ibaraki ; Ibaraki U., Grad. Sch. Sci. Eng.) ; Tsukada, Kazuaki (JAEA, Ibaraki) ; Düllmann, Christoph E (Helmholtz Inst., Mainz ; Darmstadt, GSI ; Mainz U., Inst. Kernphys.) ; Eberhardt, Klaus (Helmholtz Inst., Mainz ; Mainz U., Inst. Kernphys.) ; Eliav, Ephraim (Tel Aviv U.) ; Ichikawa, Shinichi (Nishina Ctr., RIKEN) ; Kaldor, Uzi (Tel Aviv U.) ; Kratz, Jens V (Mainz U., Inst. Kernphys.) ; Miyashita, Sunao (Hiroshima U.) ; Nagame, Yuichiro (JAEA, Ibaraki) ; Ooe, Kazuhiro (Nihon U., Tokyo) ; Osa, Akihiko (JAEA, Ibaraki) ; Renisch, Dennis (Mainz U., Inst. Kernphys.) ; Runke, Jörg (Darmstadt, GSI) ; Schädel, Matthias (JAEA, Ibaraki) ; Thörle-Pospiech, Petra (Helmholtz Inst., Mainz ; Mainz U., Inst. Kernphys.) ; Toyoshima, Atsushi (JAEA, Ibaraki) ; Trautmann, Norbert (Mainz U., Inst. Kernphys.)
Publication 2016
Number of pages 6
In: EPJ Web Conf. 131 (2016) 05001
DOI 10.1051/epjconf/201613105001
Subject category Nuclear Physics - Theory ; Nuclear Physics - Experiment
Abstract The first ionization potential (IP1) of element 103, lawrencium (Lr), has been successfully determined for the first time by using a newly developed method based on a surface ionization process. The measured IP1 value is 4.9630.080.07 eV. This value is the smallest among those of actinide elements and is in excellent agreement with the value of 4.963(15) eV predicted by state-of-the-art relativistic calculations also performed in this work. Our results strongly support that the Lr atom has an electronic configuration of [Rn]7s25f147p11/2, which is influenced by strong relativistic effects. The present work provides a reliable benchmark for theoretical calculations and also opens the way for studies on atomic properties of heavy elements with atomic number Z > 100. Moreover, the present achievement has triggered a controversy on the position of lutetium (Lu) and Lr in the Periodic Table of Elements.
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 Запись создана 2017-06-01, последняя модификация 2017-07-31


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