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Laser spectroscopy and CP-violation sensitivity of actinium monofluoride / Athanasakis-Kaklamanakis, M. (CERN ; Leuven U. ; Imperial Coll., London) ; Au, M. (CERN ; Mainz U.) ; Kyuberis, A. (Groningen U.) ; Zulch, C. (Philipps U. Marburg) ; Gaul, K. (Philipps U. Marburg ; Helmholtz Inst., Mainz ; Darmstadt, GSI ; Mainz U., Inst. Phys.) ; Wibowo, H. (York U., England) ; Skripnikov, L. (Unlisted) ; Lalanne, L. (Leuven U. ; CERN) ; Reilly, J.R. (Manchester U. ; CERN) ; Koszorus, A. (CERN ; Leuven U.) et al.
The apparent invariance of the strong nuclear force under combined charge conjugation and parity (CP) remains an open question in modern physics. [...]
arXiv:2507.05224. - 43.
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Ionization potential of radium monofluoride / Wilkins, S.G. (MIT) ; Perrett, H.A. (Manchester U.) ; Udrescu, S.M. (MIT) ; Kyuberis, A.A. (U. Groningen, VSI) ; Pašteka, L.F. (U. Groningen, VSI ; Comenius U.) ; Au, M. (CERN ; Mainz U.) ; Belošević, I. (MIT ; TRIUMF) ; Berger, R. (Philipps U. Marburg) ; Binnersley, C.L. (Manchester U.) ; Bissell, M.L. (Manchester U.) et al.
The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. [...]
arXiv:2408.14673. - 10.
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Precision spectroscopy and laser-cooling scheme of a radium-containing molecule / Udrescu, S M (MIT) ; Wilkins, S G (MIT) ; Breier, A A (Kassel U.) ; Athanasakis-Kaklamanakis, M (CERN ; Leuven U.) ; Ruiz, R F Garcia (MIT) ; Au, M (CERN ; Mainz U.) ; Belošević, I (TRIUMF) ; Berger, R (Philipps U. Marburg) ; Bissell, M L (Manchester U.) ; Binnersley, C L (Manchester U.) et al.
Molecules containing heavy radioactive nuclei are predicted to be extremely sensitive to violations of the fundamental symmetries of nature. The nuclear octupole deformation of certain radium isotopes massively boosts the sensitivity of radium monofluoride molecules to symmetry-violating nuclear properties. [...]
2024 - 14 p. - Published in : Nature Phys. 20 (2024) 202-207

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Electron correlation and relativistic effects in the excited states of radium monofluoride / ISOLDE Collaboration
We report the spectroscopy of the 14 lowest excited electronic states in the radioactive molecule radium monofluoride (RaF). The observed excitation energies are compared with fully relativistic state-of-the-art Fock-space coupled cluster (FS-RCC) calculations, which achieve an agreement of >=99.64% (within ~12 meV) with experiment for all states. [...]
arXiv:2308.14862.- 2025-03-03 - 11 p. - Published in : Nature Commun. 16 (2025) 2139 Fulltext: 2308.14862 - PDF; document - PDF PDF;

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Observation of the distribution of nuclear magnetization in a molecule / Wilkins, S.G. (MIT) ; Udrescu, S.M. (MIT) ; Athanasakis-Kaklamanakis, M. (CERN ; Leuven U.) ; Garcia Ruiz, R.F. (MIT) ; Au, M. (CERN ; Mainz U.) ; Belošević, I. (TRIUMF) ; Berger, R. (Philipps U. Marburg) ; Bissell, M.L. (Manchester U.) ; Breier, A.A. (Kassel U.) ; Brinson, A.J. (MIT) et al.
Rapid progress in the experimental control and interrogation of molecules, combined with developments in precise calculations of their structure, are enabling new opportunities in the investigation of nuclear and particle physics phenomena. [...]
arXiv:2311.04121. -
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Opportunities for Fundamental Physics Research with Radioactive Molecules / Arrowsmith-Kron, Gordon (Michigan State U.) ; Athanasakis-Kaklamanakis, Michail (CERN ; Leuven U.) ; Au, Mia (CERN ; Mainz U.) ; Ballof, Jochen (CERN ; Michigan State U.) ; Berger, Robert (Philipps U. Marburg) ; Borschevsky, Anastasia (U. Groningen, VSI) ; Breier, Alexander A. (Kassel U.) ; Buchinger, Fritz (McGill U.) ; Budker, Dmitry (Darmstadt, GSI ; UC, Berkeley) ; Caldwell, Luke (JILA, Boulder ; U. Colorado, Boulder ; Colorado U.) et al.
Molecules containing short-lived, radioactive nuclei are uniquely positioned to enable a wide range of scientific discoveries in the areas of fundamental symmetries, astrophysics, nuclear structure, and chemistry. Recent advances in the ability to create, cool, and control complex molecules down to the quantum level, along with recent and upcoming advances in radioactive species production at several facilities around the world, create a compelling opportunity to coordinate and combine these efforts to bring precision measurement and control to molecules containing extreme nuclei. [...]
arXiv:2302.02165.- 2024-07-12 - 119 p. - Published in : Rep. Prog. Phys. 87 (2024) 084301 Fulltext: PDF;

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Cool molecular highly charged ions for precision tests of fundamental physics / Zülch, Carsten (Philipps U. Marburg) ; Gaul, Konstantin (Philipps U. Marburg) ; Giesen, Steffen M. (Philipps U. Marburg) ; Garcia Ruiz, Ronald F. (MIT ; CERN) ; Berger, Robert (Philipps U. Marburg ; CERN)
Molecules and atomic highly charged ions provide powerful low-energy probes of the fundamental laws of physics: Polar molecules possess internal fields suitable to enhance fundamental symmetry violation by several orders of magnitudes, whereas atoms in high charge states can feature large relativistic effects and compressed level structures, ideally posed for high sensitivity to variations of fundamental constants. [...]
arXiv:2203.10333. - 18.
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Isotope Shifts of Radium Monofluoride Molecules / Udrescu, S.M. (MIT) ; Brinson, A.J. (MIT) ; Ruiz, R.F. Garcia (MIT ; CERN) ; Gaul, K. (Philipps U. Marburg) ; Berger, R. (Philipps U. Marburg) ; Billowes, J. (Manchester U.) ; Binnersley, C.L. (Manchester U.) ; Bissell, M.L. (Manchester U.) ; Breier, A.A. (Kassel U.) ; Chrysalidis, K. (CERN) et al.
Isotope shifts of $^{223-226,228}$Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^{2}{}{\Pi}_{1/2}\leftarrow X^{2}{}{\Sigma}^{+}$. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. [...]
arXiv:2105.10549.- 2021-07-14 - 7 p. - Published in : Phys. Rev. Lett. 127 (2021) 033001 Fulltext: 2105.10549 - PDF; PhysRevLett.127.033001 - PDF; Fulltext from publisher: PDF;

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