CERN Accelerating science

Article
Title A porous hexagonal boron nitride powder compact for the production and release of radioactive 11C
Author(s) Stegemann, S (Leuven U.) ; Ballof, J (CERN) ; Cocolios, T E (Leuven U.) ; Correia, J -G (CERN ; IST, Lisbon (main)) ; Dockx, K (Leuven U.) ; Poleshchuk, O (Leuven U.) ; Ramos, J P (Leuven U. ; CERN) ; Schell, J (CERN) ; Stora, T (CERN) ; Vleugels, J (Leuven U.)
Publication 2021
Number of pages 12
In: J. Eur. Ceramic Soc. 41 (2021) 4086-4097
DOI 10.1016/j.jeurceramsoc.2020.12.029
Subject category Health Physics and Radiation Effects
Abstract A porous pre-sintered hexagonal boron nitride powder compact was recently developed as target for the production of intense $^{11}$C beams for Positron Emission Tomography-aided hadron therapy. In a previous study, this target has been characterized regarding its operational limitations. In this work, microstructural characterization with respect to the target's grain size, porosity and pore structure, and a dedicated fractional release study from activated targets, i.e. how much $^{11}$C is extracted by a short heat treatment, is presented. Corresponding results include an average grain size of approximately 1.7(1) μm, total and open porosity of 40(5) and 21(7)%, respectively, which is mostly composed of pores with sizes ranging from 120 to 470 nm. From the measured release fraction the order of magnitude of carbon's diffusion coefficient$ D(1500 °C) = 10^{-15} - 10^{-14}$ cm$^2$ s$^{-1}$ in porous boron nitride, and a $^{11}$C extraction efficiency of about 10% at 1500 °C target temperature were estimated.
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 Journalen skapades 2022-06-17, och modifierades senast 2022-06-22